The contents are as follows.
(i) General correspondence of Caroline Eliza Grey, 1836-1890, undated (folio 1);
(ii) Draft copies of letters of Caroline Eliza Grey to Queen Victoria and Court officials, 1870-1890 (folio 101);
(iii) Family letters to the Honourable Charles Grey, 1844-1869, including a letter, 17 June 1844, of Viscount Howick concerning the political situation (folio 133);
(iv) Letters to Sybil Mary, Duchess of St Albans, from her father, the Honourable Charles Grey, and grandmother, Sybella Martha, Lady Farquhar, 1865-1869 (folio 148);
(v) Family and personal letters to Lady Victoria Alexandria Elizabeth Dawnay, 1880-1917 (folio 158);
(vi) Letters of Mary Caroline, Countess of Minto, to the Honourable Lewis Payan Dawnay, 1880-1881 (folio 225);
(vii) Election papers, chiefly printed, of the Honourable Lewis Payan Dawnay at Thirsk and Malton, 1885 (folio 236);
(viii) Family and personal letters to Louisa Jane, Countess of Antrim, 1880-1917 (folio 246);
(ix) Letter of Augusta Gieseler to the Earl of Antrim, 1932 (folio 330);
(x) Telegram of the Honourable Arthur Ralph Douglas Elliot to the Earl Grey, 1883 (folio 332).